Tomasi, C. and Vitale, V. and Tarozzi, L. (1997) Sun-photometric measurements of atmospheric turbidity variations caused by the Pinatubo aerosol cloud in the Himalayan region during the summer periods of 1991 and 1992. Il nuovo cimento C, 20 C (1). pp. 61-88. ISSN 1826-9885
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Abstract
Measurements of direct solar irradiance were taken episodically on two days of September 1990 and regularly in the summer periods from July to October 1991 and from mid-July to mid-August 1992 at the Pyramid Laboratory (5050 m a.m.s.l.) situated at the foot of Mt. Everest (Nepal), using two examples of the Volz multispectral sunphotometer, model A. These sun-photometric measurements were analysed in terms of the Bouguer-Lambert-Beer law in order to determine the values of aerosol optical thickness at the three sun-photometric window-wavelengths. Examining these spectral series in terms of the well-known Ångström formula, the best-fit values of turbidity parameters a and b were calculated with great accuracy. From the measurements taken in September 1990, we found values of the aerosol optical thickness in good agreement with the mean values of the background aerosol optical depth measured at the Mauna Loa Observatory (Hawaii) during the four-year period from 1988 to 1991. The spectral values of the aerosol optical thickness determined during the summer of 1991 show that the mean daily values of parameter b increased abruptly from about 0.06 to more than 0.16 from July 26 to 28, 1991, and then varied between 0.09 and 0.16 during the rest of the measurement period. Simultaneously, parameter a was found to decrease from more than 1.25 to 0.39 towards the end of July and to vary between 0.40 and 0.78 during September. These large variations of both atmospheric turbidity parameters have been attributed to the growth of the aerosol particles and to the consequent changes in the size distribution curve of the Pinatubo aerosol particles. Analysing the variations of the stratospheric aerosol optical depth in terms of particle polydispersions consisting of a linear combination of a background aerosol monomodal model and a bimodal model representing the Pinatubo fresh aerosol particle size distribution, the vertical mass loading of stratospheric aerosol particles was estimated to vary between 0.037 and 0.047 g m22 from July 24 to 27 and to increase to values ranging between 0.048 and 0.074 g m22 during the rest of summer 1991, presenting a mean value of (0.063 6 0.009) g m22 for the two-month period. The measurements taken in summer 1992 show that parameter b ranged between 0.08 and 0.12, while parameter a was found to vary between 0.23 and 0.73. The stratospheric aerosol depth values were analysed through a best-fit procedure based on a linear combination of a background model of small aerosol particles and a trimodal model consisting of aged volcanic aerosol particles. Following this procedure, the vertical mass loading of Pinatubo aerosol particles was found to vary between 0.043 and 0.057 g m22 during summer 1992, the mean value being evaluated as equal to (0.047 6 0.004) g m22.
| Item Type: | Article |
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| Uncontrolled Keywords: | Meteorology; particles and aerosols; atmospheric optics; atmospheric composition (atomic or molecular), chemical reactions and processes; absorption and scattering of radiation |
| Subjects: | 500 Scienze naturali e Matematica > 530 Fisica 500 Scienze naturali e Matematica > 540 Chimica e scienze connesse |
| Depositing User: | Marina Spanti |
| Date Deposited: | 09 May 2017 08:59 |
| Last Modified: | 09 May 2017 08:59 |
| URI: | http://eprints.bice.rm.cnr.it/id/eprint/11976 |
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