Excitons at room temperature in a two-dimensional quantum spin Hall insulator

Consiglio, A. (2024) Excitons at room temperature in a two-dimensional quantum spin Hall insulator. Il nuovo cimento C, 47 (5). pp. 1-6. ISSN 1826-9885

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Abstract

Both experimental techniques and theoretical methods based on density functional theory, ab-initio GW, and Bethe-Salpeter equation calculations have been employed to investigate optical resonances in the quantum spin Hall (QSH) insulator Bismuthene (a honeycomb layer of bismuth atoms) grown on a Silicon Carbide substrate. This material exhibits a direct gap of 1.3 eV at the K and K’ points, making it an excellent candidate for studying excitons in the visible and near-infrared range, even under room temperature conditions. The results, here focused on the theoretical aspects, confirm that the strong electron-hole interaction indeed has a significant impact on the optical excitations, and provide the first evidence of excitons in a 2D QSH insulator. Two main excitonic transitions are observed, with the lowest peak embedded in the single-particle direct gap, featuring a binding energy of ∼ 0.15 eV. Furthermore it is noteworthy that, in this material, both excitonic and topological features stem from the same electronic structure.

Item Type: Article
Subjects: 500 Scienze naturali e Matematica > 530 Fisica
Depositing User: Marina Spanti
Date Deposited: 09 Dec 2024 13:40
Last Modified: 09 Dec 2024 13:40
URI: http://eprints.bice.rm.cnr.it/id/eprint/23266

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